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Bressan, Giovanni 
ORCID: https://orcid.org/0000-0001-7801-8495
(2024)
Phase-Resolved fs Coherence Spectroscopy.
In: UNSPECIFIED.
(In Press)
Abstract
Here we introduce phase-resolved (PR)-FCS, derived from two-dimensional electronic spectroscopy (2DES) measurements. This yields FC spectra sensitive to amplitude and phase of vibrational, vibronic or electronic wavepackets evolving during the waiting time . Whilst 2DES beatmaps are typically amplitude normalised, PR-FC spectra retain relative intensity information, proportional to displacements between potential energy surfaces and afford a higher SNR relative to 2DES. Thus, the method provides a straightforward route to assign excited state coherence, when complex-valued 2DES data are available.
| Item Type: | Conference or Workshop Item (Poster) |
|---|---|
| Uncontrolled Keywords: | ultrafast spectroscopy,coherence,wavepackets |
| Faculty \ School: | Faculty of Science > School of Chemistry (former - to 2024) |
| Depositing User: | LivePure Connector |
| Date Deposited: | 26 Jul 2024 09:30 |
| Last Modified: | 26 Jul 2024 09:30 |
| URI: | https://ueaeprints.uea.ac.uk/id/eprint/96027 |
| DOI: |
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