Humphries, Ben S., Green, Dale ORCID: https://orcid.org/0000-0002-2549-0486, Borgh, Magnus O.
ORCID: https://orcid.org/0000-0003-4243-7051 and Jones, Garth A.
(2023)
Phonon signatures in photon correlations.
Abstract
We show that the second-order, two-time correlation functions for phonons and photons emitted from a vibronic molecule in a thermal bath result in bunching and anti-bunching (a purely quantum effect), respectively. Signatures relating to phonon exchange with the environment are revealed in photon-photon correlations. We demonstrate that cross-correlation functions have a strong dependence on the order of detection giving insight into how phonon dynamics influences the emission of light. This work offers new opportunities to investigate quantum effects in condensed-phase molecular systems.
Item Type: | Article |
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Additional Information: | 7 pages, 3 figures plus 5 pages of Supplemental material with 7 figures |
Uncontrolled Keywords: | quant-ph,physics.chem-ph |
Faculty \ School: | Faculty of Science Faculty of Science > School of Chemistry |
Related URLs: | |
Depositing User: | LivePure Connector |
Date Deposited: | 06 Feb 2023 15:30 |
Last Modified: | 09 Feb 2023 13:51 |
URI: | https://ueaeprints.uea.ac.uk/id/eprint/91045 |
DOI: |
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