Phonon signatures in photon correlations

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Humphries, Ben S., Green, Dale ORCID: https://orcid.org/0000-0002-2549-0486, Borgh, Magnus O. ORCID: https://orcid.org/0000-0003-4243-7051 and Jones, Garth A. (2023) Phonon signatures in photon correlations.

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Abstract

We show that the second-order, two-time correlation functions for phonons and photons emitted from a vibronic molecule in a thermal bath result in bunching and anti-bunching (a purely quantum effect), respectively. Signatures relating to phonon exchange with the environment are revealed in photon-photon correlations. We demonstrate that cross-correlation functions have a strong dependence on the order of detection giving insight into how phonon dynamics influences the emission of light. This work offers new opportunities to investigate quantum effects in condensed-phase molecular systems.

Item Type:	Article
Additional Information:	7 pages, 3 figures plus 5 pages of Supplemental material with 7 figures
Uncontrolled Keywords:	quant-ph,physics.chem-ph
Faculty \ School:	Faculty of Science Faculty of Science > School of Chemistry
Related URLs:	http://arxiv.org/pdf/2302.01105v1
Depositing User:	LivePure Connector
Date Deposited:	06 Feb 2023 15:30
Last Modified:	09 Feb 2023 13:51
URI:	https://ueaeprints.uea.ac.uk/id/eprint/91045
DOI:

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