Tools
Tools
Hands, Ian D., Lin, Shujie, Meech, Stephen R. 
ORCID: https://orcid.org/0000-0001-5561-2782 and Andrews, David L.
(1998)
A quantum electrodynamical treatment of second harmonic generation through phase conjugate six-wave mixing: Polarization analysis.
The Journal of Chemical Physics, 109 (24).
ISSN 0021-9606
Preview |
PDF (109)
- Published Version
Download (208kB) | Preview |
Abstract
The theory underlying a six-wave mixing experiment is developed using the methods of molecular quantum electrodynamics. This general theory allows the intensity of the second harmonic radiation generated by the six-wave process to be found for arbitrary arrangements of the generating laser beams. Several different polarization geometries are treated in detail, and comparison is made to experiments performed using near-resonant conditions. The agreement is good in all cases and allows detailed information pertaining to the six-wave tensor to be extracted. The information thus obtained provides evidence of a marked departure from Kleinman symmetry.
| Item Type: | Article |
|---|---|
| Faculty \ School: | Faculty of Science > School of Chemistry (former - to 2024) |
| UEA Research Groups: | Faculty of Science > Research Groups > Physical and Analytical Chemistry (former - to 2017) Faculty of Science > Research Groups > Chemistry of Light and Energy Faculty of Science > Research Groups > Centre for Photonics and Quantum Science |
| Depositing User: | Pure Connector |
| Date Deposited: | 18 Jan 2016 17:02 |
| Last Modified: | 24 Sep 2024 11:32 |
| URI: | https://ueaeprints.uea.ac.uk/id/eprint/56500 |
| DOI: | 10.1063/1.477757 |
Downloads
Downloads per month over past year
Actions (login required)
 |
View Item |