Global 3D model analysis of the seasonal cycle of atmospheric carbonyl sulfide: Implications for terrestrial vegetation uptake

Suntharalingam, Parvadha, Kettle, A. J., Montzka, S. M. and Jacob, D. J. (2008) Global 3D model analysis of the seasonal cycle of atmospheric carbonyl sulfide: Implications for terrestrial vegetation uptake. Geophysical Research Letters, 35 (19). L19801. ISSN 1944-8007

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Abstract

We use a global 3-D simulation of atmospheric carbonyl sulfide (COS) to interpret observations at a network of surface sites. We aim to identify the primary factors underlying observed seasonal variations and to constrain COS uptake by terrestrial vegetation. Model simulations are based on a recent estimate of global COS fluxes, with closure between sources and sinks. We find that the dominant influences on seasonal variation of COS are terrestrial vegetation uptake in the northern extratropics, and ocean fluxes in the southern extratropics. Simulations underestimate the amplitude of the observed seasonal cycle in the northern hemisphere, particularly at terrestrial sites, indicating that COS uptake by terrestrial vegetation has been underestimated in recent budgets. Fitting the observed seasonal variation at northern hemisphere sites in the model requires a doubling of the global vegetation sink to ~490 Gg S y-1, while fitting the southern hemisphere data suggests a reduction of ~50 Gg S y-1 in the southern extratropical ocean source. Balancing these changes in COS fluxes requires an additional source (~235 Gg S y-1, equivalent to 40% of identified sources) missing from present budget estimates. Discrepancies between annual mean observations and simulated concentrations, derived from our best estimates of seasonal fluxes, are largest in the tropics, suggesting an underestimate of COS sources at these latitudes.

Item Type:	Article
Faculty \ School:	Faculty of Science > School of Environmental Sciences
UEA Research Groups:	Faculty of Science > Research Groups > Centre for Ocean and Atmospheric Sciences Faculty of Science > Research Groups > Marine and Atmospheric Sciences (former - to 2017) Faculty of Science > Research Groups > Atmospheric Chemistry (former - to 2018) Faculty of Science > Research Groups > Climate, Ocean and Atmospheric Sciences (former - to 2017)
Depositing User:	Rosie Cullington
Date Deposited:	02 Mar 2011 09:42
Last Modified:	29 Jan 2025 11:01
URI:	https://ueaeprints.uea.ac.uk/id/eprint/25518
DOI:

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