Enhanced output from biohybrid photoelectrochemical transparent tandem cells integrating photosynthetic proteins genetically modified for expanded solar energy harvesting

Ravi, Sai Kishore, Yu, Zhimeng, Swainsbury, David J. K., Ouyang, Jianyong, Jones, Michael R. and Tan, Swee Ching (2017) Enhanced output from biohybrid photoelectrochemical transparent tandem cells integrating photosynthetic proteins genetically modified for expanded solar energy harvesting. Advanced Energy Materials, 7 (7). ISSN 1614-6832

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Abstract

A transparent biohybrid photoelectrochemical tandem cell is developed by employing optically-complementary variants of a photosynthetic protein in a stacked tandem architecture that utilizes a conductive polymer, poly(3,4-ethylenedioxythiophene):polystyrene sulfonate (PEDOT:PSS), as a transparent counter electrode. The tandem design demonstrates the photocurrent enhancement by complementary absorption of two naturally-occurring red and green versions of a bacterial Reaction center/Light Harvesting protein (RC-LH1) that vary in the type of light harvesting carotenoid feeding the central reaction center module with excited state energy. The use of PEDOT:PSS electrode results in a 12-fold improvement in photocurrent compared to that achievable with Platinum.

Item Type: Article
Additional Information: Funding Information: D.J.K.S. and M.R.J. acknowledge the support from the Biotechnology and Biological Sciences Research Council of the UK (project BB/I022570/1). S.K.R. and S.C.T. acknowledge the financial support from MOE AcRF 1 (R-284-000-134-112 and R-284-000-129-133).
Uncontrolled Keywords: biophotovoltaics,genetic modification,pedot:pss,photosynthetic proteins,transparent tandem solar cells,renewable energy, sustainability and the environment,materials science(all),sdg 7 - affordable and clean energy ,/dk/atira/pure/subjectarea/asjc/2100/2105
Faculty \ School: Faculty of Science > School of Biological Sciences
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Depositing User: LivePure Connector
Date Deposited: 17 Aug 2022 12:32
Last Modified: 22 Oct 2022 07:55
URI: https://ueaeprints.uea.ac.uk/id/eprint/87378
DOI: 10.1002/aenm.201601821

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