Stratospheric ozone changes under solar geoengineering:Implications for UV exposure and air quality

Nowack, Peer Johannes, Abraham, Nathan Luke, Braesicke, Peter and Pyle, John (2016) Stratospheric ozone changes under solar geoengineering:Implications for UV exposure and air quality. Atmospheric Chemistry and Physics, 16 (6). pp. 4191-4203. ISSN 1680-7316

[img]
Preview
PDF (Published_Version) - Published Version
Available under License Creative Commons Attribution.

Download (2MB) | Preview

Abstract

Various forms of geoengineering have been proposed to counter anthropogenic climate change. Methods which aim to modify the Earth's energy balance by reducing insolation are often subsumed under the term solar radiation management (SRM). Here, we present results of a standard SRM modelling experiment in which the incoming solar irradiance is reduced to offset the global mean warming induced by a quadrupling of atmospheric carbon dioxide. For the first time in an atmosphere–ocean coupled climate model, we include atmospheric composition feedbacks for this experiment. While the SRM scheme considered here could offset greenhouse gas induced global mean surface warming, it leads to important changes in atmospheric composition. We find large stratospheric ozone increases that induce significant reductions in surface UV-B irradiance, which would have implications for vitamin D production. In addition, the higher stratospheric ozone levels lead to decreased ozone photolysis in the troposphere. In combination with lower atmospheric specific humidity under SRM, this results in overall surface ozone concentration increases in the idealized G1 experiment. Both UV-B and surface ozone changes are important for human health. We therefore highlight that both stratospheric and tropospheric ozone changes must be considered in the assessment of any SRM scheme, due to their important roles in regulating UV exposure and air quality

Item Type: Article
Uncontrolled Keywords: atmospheric science ,/dk/atira/pure/subjectarea/asjc/1900/1902
Related URLs:
Depositing User: LivePure Connector
Date Deposited: 11 Feb 2020 05:34
Last Modified: 24 Nov 2020 01:33
URI: https://ueaeprints.uea.ac.uk/id/eprint/74082
DOI: 10.5194/acp-16-4191-2016

Actions (login required)

View Item View Item